| Character | How to unlock
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|---|
| A.I.M. Agent | Complete Level 10: That Sinking Feeling.
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| Abomination | Complete Level 4: Rock up at the Lock up.
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| Absorbing Man | Collect his token in Industrial District.
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| Agent Coulson | Complete Bonus Level: Tabloid Tidy UP.
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| Aldrich Killian | Complete Level 5: Rebooted, Resuited.
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| Ant-Man | Collect his token in the Industrial District.
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| Archangel | Collect his token south of the X-Mansion, to the south of giant billboard.
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| Arnim Zola | Complete Level 6: Red Head Detention.
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| Aunt May | Complete Deadpool's 3 missions.
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| Beast | Complete Level 8: Juggernauts and Crosses.
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| Beetle | Collect his token a block east of the central park lake.
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| Black Bolt | Complete Gambit's first mission.
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| Black Cat | Collect her token below Lady Liberty on the map in a cat pet shop (requires Spider Man to unlock).
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| Black Panther | Complete his 3 missions.
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| Black Widow | Complete Level 3: Exploratory Laboratory.
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| Blade | Complete his 3 missions.
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| Blob | Complete Bonus Level: Put Up Your Dukes.
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| Bullseye | Collect his token in Slums District.
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| Captain America | Complete Level 2: Times Square Off.
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| Captain America (Comics) | Complete Bonus Level: The Brick Apple.
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| Captain Britain | Complete Bonus Level: The Brick Apple.
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| Carnage | Collect his token in Residential District.
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| Colossus | Collect Colossus token in the front right courtyard of the X-Mansion.
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| Cyclops | Complete Level 8: Juggernauts and Crosses.
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| Cyclops (Astonishing) | Taxi the character in the Financial District to his destination, then collect his token.
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| Damage Control | Put the out fires on the SHIELD Helicarrier deck with the water gun.
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| Daredevil | Complete Bonus Level: Feeling Frisky.
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| Deadpool | Collect all Deadpool Red Bricks.
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| Doctor Doom | Complete Level 14: "A Doom with a View".
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| Doctor Octopus | Complete Level 2: Times Square Off.
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| Doctor Octopus (Ultimate) | Complete Bonus Level: Tabloid Tidy UP.
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| Doctor Strange | Complete Bonus Level: Stranger Danger.
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| Doombot | Complete Level 9: Doctor in the House.
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| Doombot (V-Series) | Complete Level 14: "A Doom with a View".
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| Drax the Destroyer | Complete the story, then complete his 3 missions.
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| Electro | Complete Bonus Level: A Shock Withdrawal.
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| Electro (Ultimate) | Taxi the character in front of the Oscorp building to her destination, then collect his token.
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| Elektra | Collect her token in Slums District.
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| Emma Frost | Complete a mission Professor X hands out.
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| Frost Giant | Complete Level 7 - Bifrosty Reception.
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| Galactus (Minifig) | Complete Level 15: The Good, the Bad and the Hungry.
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| Gambit | Complete his 3 missions.
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| Gamora | Complete the story, then complete the first mission you get from Drax.
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| Ghost Rider | Complete Bonus Level: Stunt Show Surprise.
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| Green Goblin | Complete Level 9: Doctor in the House.
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| Green Goblin (Ultimate) | Collect his token in Bonus Level: Thrill of the Chess.
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| Groot | Complete the story, then complete his 3 missions.
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| Gwen Stacy | Complete "Mission 47" for Drax.
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| H.E.R.B.I.E. | Complete Level 2: Times Square Off.
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| Havok | Collect his token in the Forest District.
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| Hawkeye | Complete Level 3: Exploratory Laboratory.
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| Heimdall | Complete his 3 missions.
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| Howard the Duck | Complete Bonus Level: Nuff Said.
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| Hulk | Complete Level 1: Sand Central Station.
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| Human Torch | Complete Level 6: Red Head Detention.
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| Hydra Agent | Collect his token in the Forest District.
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| Iceman | Complete Level 8: Juggernauts and Crosses.
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| Invisible Woman | Complete Level 9: Doctor in the House.
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| Invisible Woman (Future Foundation) | Collect her token in Bonus Level: Stranger Danger.
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| Iron Fist | Complete race mission with Blade, then win the fight with ice dudes in the next Blade mission.
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| Iron Man (Heroic Age) | Complete Bonus Level: New York Event.
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| Iron Man (Hulkbuster) | Land on "S" sign landing platform, then take out all the airvents that are all around the "S" sign.
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| Iron Man MK I | Complete Level 5: Rebooted, Resuited.
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| Iron Man MK VI | Complete Level 1: Sand Central Station.
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| Iron Man MK VII | Complete Bonus Level: House Party Protocol.
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| Iron Man MK XLVII | Complete Level 5: Rebooted, Resuited.
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| Iron Man MK XVII | Complete Bonus Level: House Party Protocol.
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| J. Jonah Jameson | Complete Bonus Level: Tabloid Tidy Up.
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| Jean Grey | Complete Level 8: Juggernauts and Crosses.
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| Juggernaut | Complete Level 8: Juggernauts and Crosses.
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| Kingpin | Complete Bonus Level: Feeling Frisky.
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| Kingpin Henchman | Collect his token in Bonus Level: Feeling Frisky.
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| Kraven the Hunter | Shoot the five targets next to the Godzilla-looking icon at the Central Park.
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| Kurse | Defeat him in battle near Roxxon Power Station, then collect his token.
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| Lady Liberty (Minifig) | Complete Level 11: Taking Liberties.
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| Laufey | Complete Bonus Level: Bro-tunheim.
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| Loki | Complete Level 15: The Good, the Bad and the Hungry.
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| M.O.D.O.K. | Complete Level 10 - That Sinking Feeling.
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| Magneto | Complete Level 13 - Magnetic Personality.
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| Magneto Acolyte | Complete Level 13: Magnetic Personality.
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| Malekith | Complete Bonus Level: Bro-tunheim.
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| Mandarin (Film) | Collect his token in Bonus Level: Stunt Show Surprise.
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| Maria Hill | Complete her 3 missions on the Helicarrier.
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| Mary Jane Watson | Collect her token in the Residential District.
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| Mister Fantastic | Complete Level 2: Times Square Off.
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| Mister Fantastic (Future Foundation) | Defeat Ghost Rider in a race starting in West Harlem.
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| Moon Knight | Collect his token in Bonus Level: A Shock Withdrawl.
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| Ms. Marvel | Collect her token in Bonus Level: 'Nuff Said.
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| Mysterio | Complete Bonus Level: Thrill of the Chess.
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| Mystique | Complete Level 12: Rapturous Rise.
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| Nick Fury | Complete Level 9: Doctor in the House.
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| Nightmare | Complete Bonus Level: Stunt Show Surprise.
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| Nova | Complete foot race mission with him at the east of the giant Godzilla icon in the Central Park.
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| Pepper Potts | Complete Black Panther's first mission.
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| Phoenix | Complete Bonus Level: Put up your Dukes.
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| Polaris | Complete Bonus Level: Thrill of the Chess.
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| Power Man | Collect his token in Yorkville District.
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| Professor Xavier | Complete his 3 missions behind the X-Mansion.
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| Psylocke | Complete all Captain Britain missions.
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| Punisher | Complete his 3 missions.
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| Pyro | Complete Level 8: Juggernauts and Crosses.
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| Red Hulk | Defeat Red Hulk in battle, then collect his token.
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| Red Skull | Complete Level 6: Red Head Detention.
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| Rescue | Complete Black Panther's second mission.
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| Rhino | Complete Level 12: Rapturous Rise.
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| Rocket Raccoon | Complete his 3 missions.
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| Ronan the Accuser | Find hidden path behind the statue south of his icon.
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| Roxxon Agent | Complete Level 1: Sand Central Station.
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| S.H.I.E.L.D. Agent | Collect his token on the Helicarrier.
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| Sabretooth | Complete Level 4: Rock Up at the Lock Up.
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| Sandman | Complete Level 1: Sand Central Station.
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| Sandman Goon | Collect his token directly east of the Lizard House near the water.
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| Sentinal (Minifig) | Defeat the Sentinal, then collect its token.
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| She-Hulk | Collect her token in the Scrapyard.
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| Shocker | Complete Bonus Level: A Shock Withdrawl.
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| Silver Samurai | Collect his token in the Industrial District.
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| Silver Surfer | Complete his 3 missions.
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| Spider-Man | Complete Level 1: Sand Central Station.
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| Spider-Man (Future Foundation) | Defeat Ghost Rider in a race in the Dockyard.
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| Spider-Woman | Collect her token west of the park on the southern most part of the island.
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| Squirrel Girl | Collect her token in the Dockyard.
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| Stan Lee | Rescue all 50 Stan Lee in Peril.
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| Star-Lord | Complete his 3 missions.
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| Storm | Complete Level 8: Juggernauts and Crosses.
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| Super-Skrull | Collect his token in the Upper East Side.
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| Superior Spider-Man | Skydive off the Empire State Building, falling through the rings of studs. You will collect this token near the ground.
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| Symbiote Scientist | Complete Level 3: Exploratory Laboratory.
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| Symbiote Scientist (Hazmat) | Complete Level 3: Exploratory Laboratory.
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| Taskmaster | Collect his token on a platform above the clouds east of Liberty Island.
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| The Destroyer (Minifig) | Complete Level 7: Bifrosty Reception.
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| The Leader | Collect his Token near Fisk Tower.
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| The Mandarin | Complete Level 5: Rebooted, Resuited.
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| Thing | Complete Level 9: Doctor in the House.
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| Thing (Future Foundation) | Collect his token in Bonus Level: Reptillian Ruckus.
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| Thor | Complete Level 7: Bifrosty Reception.
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| Thor (Classic) | Collect his token in Bonus Level: Bro-tunheim.
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| Toad | Complete his 3 missions.
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| Tony Stark | Complete Level 5: Rebooted, Resuited.
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| Tony Stark (Underwear) | Complete Level 4: Rock up at the Lock up.
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| Union Jack | Complete Bonus Level: The Brick Apple.
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| Venom | Complete Level 3: Exploratory Laboratory.
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| Viper | Collect his token in Central Park.
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| Vulture | Complete Bonus Level: 'Nuff Said.
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| War Machine | Complete Bonus Level: House Party Protocol.
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| Wasp | Collect his token one block south of the Oscorp Building.
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| Whiplash | Collect his token in Yorkville.
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| Wizard | Collect his token on the Baxter Building.
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| Wolverine | Complete Level 4: Rock up at the Lock up.
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| Wolverine (Cowl) | Collect his token in Bonus Level: Put up your Dukes.
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| Achievement | How to unlock
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|---|
| A Doom with a View | Complete Level 14 - A Doom with a View.
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| Alter Ego | Perform all big LEGO figure transformations.
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| Avengers Assembled | Collect all Avengers characters in the game (Single Player).
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| Bad Luck? | Unlock Black Cat (Single Player).
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| Bifrosty Reception | Complete Level 7 - Bifrosty Reception.
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| Billionaire Philanthropist | Collect 1,000,000,000 studs (Single Player).
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| Brotherhood | Collect all traditionally evil mutants (Single Player).
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| Can't Hurt Me Bub | Regenerate as Wolverine.
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| Cosplay | Create a custom character.
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| Doctor in the House | Complete Level 9 - Doctor in the House.
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| Don't I Know You? | Team up Captain America with Human Torch (Co-op).
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| Exploratory Laboratory | Complete Level 3 - Exploratory Laboratory.
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| Falling... with Style | Complete first Helicarrier skydive.
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| Fastball Special | Perform a special throwing move as Colossus on Wolverine.
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| Guardians of the Galaxy | Unlock all the Guardians of the Galaxy (Single Player).
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| I Am Iron Man | Collect all Iron Man armors (Single Player).
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| I'm Always Angry! | Transform into the Hulk 50 times.
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| It's Clobberin' Time! | Defeat 100 enemies as the Thing.
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| It's Me Time! | Read a comic in Deadpool's room on the Helicarrier.
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| Juggernauts and Crosses | Complete Level 8 - Juggernauts and Crosses.
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| Magnetic Personality | Complete Level 13 - Magnetic Personality.
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| Menace of Magneto | Drive to the Baxter Building as Magneto in the Magneto Mobile.
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| Post-Credit Party | Complete House Party Protocol.
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| Puny God | Perform Hulk's special move on Loki.
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| Rapturous Rise | Complete Level 12 - Rapturous Rise.
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| Really? | Collect Howard the Duck (Single Player).
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| Rebooted, Resuited | Complete Level 5 - Rebooted, Resuited.
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| Red Head Detention | Complete Level 6 - Red Head Detention.
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| Road Rage | Destroy 100 vehicles in the Manhattan hub.
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| Rock up at the Lock up | Complete Level 4 - Rock up at the Lock up.
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| Sand Central Station | Complete Level 1 - Sand Central Station.
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| Sinister Six | Collect Doc Ock, Sandman, Mysterio, Kraven the Hunter, Electro and Vulture (Single Player).
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| Stan's Soapbox | Turn into Stan Hulk.
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| Stan-tastic | Rescue Stan Lee from every peril (Single Player).
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| Taking Liberties | Complete Level 11 - Taking Liberties.
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| That Sinking Feeling | Complete Level 10 - That Sinking Feeling.
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| The Good, the Bad and the Hungry | Complete Level 15 - The Good, the Bad and the Hungry.
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| The Toast of Croydon | Create a character called 'Trevor' in the character customizer.
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| This Is fantastic! | First time turning Mister Fantastic into a teapot.
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| Times Square Off | Complete Level 2 - Times Square Off.
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| To Me, My X-Men | Collect all traditionally heroic mutants (Single Player).
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| Ultimate True Believer | Unlock all True Believers (Single Player).
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| Welcome to Level 7 | Play as Agent Coulson.
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| You Win a No-Prize! | Complete game 100% (Single Player).
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| Zoo Believer | Unlock all animal-themed characters (Single Player).
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